@ The University of Oklahoma

Category: New Publications Page 1 of 2

New paper on reservoir CH4 emission published in Water Research

Our new paper, “Methane dynamics
altered by reservoir operations in a typical tributary of the Three Gorges Reservoir
“, is published in Water Research (IF: 11.4).

The paper and its supplement can be downloaded at https://www.sciencedirect.com/science/article/pii/S0043135424010625.

Authors: Jia Liu, Fei Xue, Xiaojuan Guo, Zhengjian Yang, Manchun Kang, Min Chen, Daobin Ji, Defu Liu, Shangbin Xiao, and Chenghao Wang

Abstract: Substantial nutrient inputs from reservoir impoundment typically increase sedimentation rate and primary production. This can greatly enhance methane (CH4) production, making reservoirs potentially significant sources of atmospheric CH4. Consequently, elucidating CH4 emissions from reservoirs is crucial for assessing their role in the global methane budget. Reservoir operations can also influence hydrodynamic and biogeochemical processes, potentially leading to pronounced spatiotemporal heterogeneity, especially in reservoirs with complex tributaries, such as the Three Gorges Reservoir (TGR). Although several studies have investigated the spatial and temporal variations in CH4 emissions in the TGR and its tributaries, considerable uncertainties remain regarding the impact of reservoir operations on CH4 dynamics. These uncertainties primarily arise from the limited spatial and temporal resolutions of previous measurements and the complex underlying mechanisms of CH4 dynamics in reservoirs. In this study, we employed a fast-response automated gas equilibrator to measure the spatial distribution and seasonal variations of dissolved CH4 concentrations in XXB, a representative area significantly impacted by TGR operations and known for severe algal blooms. Additionally, we measured CH4 production rates in sediments and diffusive CH4 flux in the surface water. Our multiple campaigns suggest substantial spatial and temporal variability in CH4 concentrations across XXB. Specifically, dissolved CH4 concentrations were generally higher upstream than downstream and exhibited a vertical stratification, with greater concentrations in bottom water compared to surface water. The peak dissolved CH4 concentration was observed in May during the drained period. Our results suggest that the interplay between aquatic organic matter, which promotes CH4 production, and the dilution process caused by intrusion flows from the mainstream primarily drives this spatiotemporal variability. Importantly, our study indicates the feasibility of using strategic reservoir operations to regulate these factors and mitigate CH4 emissions. This eco-environmental approach could also be a pivotal management strategy to reduce greenhouse gas emissions from other reservoirs.

DOI: https://doi.org/10.1016/j.watres.2024.122163

This image has an empty alt attribute; its file name is 1-s2.0-S0043135424010625-gr6_lrg-scaled.jpg

Fig. 6. Conceptual diagram of CH4 dynamics in Xiangxi Bay under the operations of the Three Gorges Reservoir. The light blue area represents inflow from upstream of XXR, while the dark blue area represents flow from the mainstream. Orange and green circles along the riverbed represent terrestrial and aquatic OM, respectively. Solid green circles near the water surface represent algae.

New paper on benzene emissions published in Atmospheric Environment X

Our new paper, “A modeling framework to assess fenceline monitoring and self-reported upset emissions of benzene from multiple oil refineries in Texas“, is published in Atmospheric Environment X (IF: 3.8).

The paper and its supplement can be downloaded at https://www.sciencedirect.com/science/article/pii/S2590162124000480.

Authors: Qi Li, Lauren Padilla, Tammy Thompson, Shuolin Xiao, Elizabeth Mohr, Xiaohe Zhou, Nino Kacharava, Yuanfeng Cui, and Chenghao Wang

Abstract: Benzene as one type of hazardous air pollutants (HAPs) is produced by industrial production processes and/or emitted during upset events caused by man-made or natural accidents. Although upset emissions of benzene can be a significant contributor to the total emission, it is still challenging to quantify. This study first develops a fast modeling framework using obstacle-resolving computational fluid dynamics modeling to compare the modeled within-facility-scale passive pollutant dispersion with the observed levels based on self-reported emissions for fourteen facilities in Texas, United States. Results of numerical simulations demonstrate that neglecting the obstacle effect can underpredict (overpredict) the near-(far-)field concentrations for a low source. For a source located above obstacles, underprediction occurs at all distances. The diagnostic framework is applied to 107 self-reported upset emission events for fourteen petroleum refineries in Texas from year 2019–2022. Considering different metrics across all events, it can be concluded that the modeled concentrations based on self-reported emissions likely underpredict the observed concentration increments. Depending on the possible source height, the median factor of underprediction ranges from 3 to 95 based on the average-plume metric. The agreement between model and observation is better for events characterized by high emission amounts and rates, which also correspond to high observed concentration increments. Overall, the research highlights the importance of considering obstacles and demonstrates the potential application of the current approach as an efficient diagnostic method for self-reported upset emissions using fenceline observations of HAPs.

DOI: https://doi.org/10.1016/j.aeaoa.2024.100281

Fig. 2. Normalized concentrations
for cases without and with obstacles for horizontal plane at z = 2 m.
The wind direction is zero degree, the obstacle geometry is sparse-low. The obstacles, i.e., the “white-bars” are 100 m × 100 m and the gap between, d, is 200 m in this example. The planar location of the source is indicated by the blue star in Fig. 1a; the top, middle, to bottom rows show cases with source heights corresponding to low, medium, and high as indicated in Fig. 1b. (a), (c), (e): C’LES for cases without obstacles with source heights zs low, medium and high. (b), (d), (f): C’LES for case with sparse-low obstacles with source heights zs low, medium and high.

Open postdoctoral researcher positions in urban air quality and GHG modeling

The School of Meteorology and the Center for Analysis and Prediction of Storms at the University of Oklahoma invite applications for two fully funded full-time Postdoctoral Researcher positions focused on the modeling of air quality and/or greenhouse gases (GHGs) in the urban environment. Areas of focus include but are not limited to:

  • Development of new or improved numerical parameterization schemes
  • Spatial and temporal characterization of air pollution (e.g., ozone and particulate matter) and GHGs
  • Assessment of mitigation strategies to reduce air pollutants and GHG emissions

Both positions are based in Norman, OK, and will be working with Dr. Chenghao Wang and Dr. Xiao-Ming Hu.

Salary will be commensurate with the applicant’s experience. Full-time employment comes with OU research staff benefits, including generous paid leave, health insurance, and retirement savings plans. The successful candidates will work in the National Weather Center, with numerous opportunities to collaborate with world-leading academic and operational partners both on and off campus, such as the Center for Analysis and Prediction of Storms (CAPS) and National Center for Atmospheric Research (NCAR). The University of Oklahoma and City of Norman offer a vibrant college town atmosphere with numerous recreational and cultural activities. Norman is just 20 miles away from Oklahoma City, which provides all the amenities of a larger city. Norman also has a low cost of living compared to most cities in the U.S.

Qualifications: Applicants must have earned a Ph.D. in Atmospheric Sciences, Engineering, Earth Science, Computer Science, or a closely related field by the time of appointment. Candidates should have demonstrated experience with numerical 3D air quality models, such as WRF-Chem, CMAQ, HYSPLIT, GEOS-Chem, and LES models, be proficient in programming languages commonly used in models (Fortran) and data analytics (MATLAB, Python, R, or NCL), and possess strong oral and written communication skills, evidenced by their publication record and presentations at scientific meetings.

Application Instructions

Applicants are encouraged to apply as soon as possible. To apply, interested individuals should submit electronically:

(1) A cover letter explaining their interest and qualifications for the position.

(2) A curriculum vitae.

(3) Two to three representative publications (journal articles, conference papers, or preprints).

(4) Contact information for three professional references.

Please submit your application through http://apply.interfolio.com/150611 by Sep 30, 2024. Applications will be reviewed as received and will continue until the positions are filled. For questions regarding these two positions, please contact Dr. Chenghao Wang (chenghao.wang@ou.edu) or Dr. Xiao-Ming Hu (xhu@ou.edu).

Dr. Wang received the NASA Early Career Investigator Grant

Dr. Wang was recently awarded the NASA Early Career Investigator Grant titled “Compound Heat and Ozone Pollution Episodes in the Urban Environment: Dynamics, Mechanism, and Mitigation with Nature-Based Solutions”.

See OU News here: https://www.ou.edu/news/articles/2024/july/researcher-receives-nasa-funding-to-study-ozone-pollution.

New paper on urban irrigation published in Nature Communications

Our new paper, “The potential of urban irrigation for counteracting carbon-climate feedback“, is published in Nature Communications (IF: 16.6).

The paper and its supplement can be downloaded at https://www.nature.com/articles/s41467-024-46826-3.

Authors: Peiyuan Li, Zhi-Hua Wang, and Chenghao Wang

Abstract: Global climate changes, especially the rise of global mean temperature due to the increased carbon dioxide (CO2) concentration, can, in turn, result in higher anthropogenic and biogenic greenhouse gas emissions. This potentially leads to a positive loop of climate–carbon feedback in the Earth’s climate system, which calls for sustainable environmental strategies that can mitigate both heat and carbon emissions, such as urban greening. In this study, we investigate the impact of urban irrigation over green spaces on ambient temperatures and CO2 exchange across major cities in the contiguous United States. Our modeling results indicate that the carbon release from urban ecosystem respiration is reduced by evaporative cooling in humid climate, but promoted in arid/semi-arid regions due to increased soil moisture. The irrigation-induced environmental co-benefit in heat and carbon mitigation is, in general, positively correlated with urban greening fraction and has the potential to help counteract climate–carbon feedback in the built environment.

DOI: https://doi.org/10.1038/s41467-024-46826-3

Fig. 2: Governing mechanisms on carbon exchange of urban greenery. a A diagram showing carbon exchange of plants in the built environment with UHI, higher background CO2 concentration, and management (irrigation). b Irrigation-induced change of urban gross primary productivity (dGPPu), led by decrease of air temperature and increase of soil water content. c Irrigation-induced change of urban ecosystem respiration (dRu), led by decrease of soil temperature and increase of soil water content. d Irrigation-induced change of urban net ecosystem exchange (dNEEu), resulting from the combinations of dGPPu and dRu. e Urban ecosystem respiration as a function of soil temperature and soil water content. The light gray lines in b–d show all possible combinations lead to various types of outcomes. The black solid lines indicate pathway to the strong co-benefit effect. The red dashed lines indicate the pathway to the strong tradeoff effect. Circles in (e) indicate the average Ru before (hollow) and after (solid) irrigation. Arrows indicate the direction of change.

New paper on the cooling dynamics of urban vegetation published in Remote Sensing of Environment

Our new paper, “Enhanced observations from an optimized soil-canopy-photosynthesis and energy flux model revealed evapotranspiration-shading cooling dynamics of urban vegetation during extreme heat“, is published in Remote Sensing of Environment (IF: 13.5).

The paper and its supplement can be downloaded at https://www.sciencedirect.com/science/article/pii/S0034425724001093. The Share Link to download a copy is https://authors.elsevier.com/c/1ikad7qzT3Dj5 (valid through Apr 30, 2024).

Authors: Zhaowu Yu, Jiaqi Chen, Jike Chen, Wenfeng Zhan, Chenghao Wang, Wenjuan Ma, Xihan Yao, Siqi Zhou, Kai Zhu, and Ranhao Sun

Abstract: Previous studies on the cooling of urban vegetation mainly focused on its transpiration or shading effect separately, neglecting to explore the combined evapotranspiration-shading cooling. Further, accurate quantification of evapotranspiration-shading cooling remains challenging due to heterogeneity of urban landscapes, which limits understanding of its high-resolution spatiotemporal patterns. Here, we integrate high-precision remote sensing data and the Soil-Canopy-Observations of Photosynthesis and Energy Fluxes (SCOPE) model to propose an optimized quantitative approach. The approach was used to investigate changes in evapotranspiration-shade cooling during extreme heat. Taking Shanghai metropolitan as case, the results show: (1) The cooling capacity of urban vegetation in nighttime (18:00–6:00) is enhanced during extreme heat, which is attributed to accumulated effect of shading and enhanced evapotranspiration due to elevated vapor-pressure deficit. (2) In densely built-up areas with limited vegetation, there is a significant lack of thermal regulation, especially in the early morning (7:00) and late evening (17:00), thus exacerbating thermal stress. (3) At midday (11:00–13:00) there was a slight decrease in evaporative cooling, probably caused by the behaviour of the stomatal closure at high temperatures. Concurrently, high radiation causes the shading effect of vegetation to become more prominent, amplifying the cooling contrast between areas with dense and sparse vegetation cover. Moreover, the study also highlights that grassland with >50% cover can provide cooling effects similar to that of forest land. Overall, our study not only enhances the understanding of urban vegetation’s cooling effects but also underscores the importance of strategic urban vegetation planning in mitigating urban heat, particularly under the escalating frequency and intensity of heat waves.

DOI: https://doi.org/10.1016/j.rse.2024.114098

Fig. 5. Distribution patterns of urban vegetation evapotranspiration-induced cooling at typical moments of the daily cycle during heat waves in Shanghai.

New paper on urban causal interactions under heat waves published in npj Urban Sustainability

Our new paper, “Megacities are causal pacemakers of extreme heatwaves“, is published in npj Urban Sustainability.

The paper and its supporting information can be downloaded at https://www.nature.com/articles/s42949-024-00148-x.

Authors: Xueli Yang, Zhi-Hua Wang, Chenghao Wang, and Ying-Cheng Lai

Abstract: Global climate change has been shown to cause longer, more intense, and frequent heatwaves, of which anthropogenic stressors concentrated in urban areas are a critical contributor. In this study, we investigate the causal interactions during heatwaves across 520 urban sites in the U.S. combining complex network and causal analysis. The presence of regional mediators is manifest in the constructed causal networks, together with long-range teleconnections. More importantly, megacities, such as New York City and Chicago, are causally connected with most of other cities and mediate the structure of urban networks during heatwaves. We also identified a significantly positive correlation between the causality strength and the total populations in megacities. These findings corroborate the contribution of human activities e.g., anthropogenic emissions of greenhouse gases or waste heat, to urban heatwaves. The emergence of teleconnections and supernodes are informative for the prediction and adaptation to heatwaves under global climate change.

DOI: https://doi.org/10.1038/s42949-024-00148-x

Fig. 6. Comparison of causality (outdegree) with two population metrics for 53 large U.S. cities with a population over 200,000 during the 2020 heatwave event (July 18-22). a, b For population totals, and c, d are for population density. The top panel shows comparison maps of the causal outdegree (triangular markers) and population metrics: population totals in a and population density in c, with sizes represented by gray shaded circles. The bottom panel represents the log-log correlation between the causal outdegree and population metrics: population totals in b and population density in d and causality, with sizes represented by colored circles.

New paper on extreme fire weather published in Scientific Reports

Our new paper, “Extreme fire weather in Chile driven by climate change and El Niño–Southern Oscillation (ENSO)“, is published in Scientific Reports (IF: 4.6).

The paper and its supporting information can be downloaded at https://www.nature.com/articles/s41598-024-52481-x.

Authors: Raúl R. Cordero, Sarah Feron, Alessandro Damiani, Jorge Carrasco, Cyrus Karas, Chenghao Wang, Clarisse T. Kraamwinkel, and Anne Beaulieu

Abstract: A string of fierce fires broke out in Chile in the austral summer 2023, just six years after the record-breaking 2017 fire season. Favored by extreme weather conditions, fire activity has dramatically risen in recent years in this Andean country. A total of 1.7 million ha. burned during the last decade, tripling figures of the prior decade. Six of the seven most destructive fire seasons on record occurred since 2014. Here, we analyze the progression during the last two decades of the weather conditions associated with increased fire risk in Central Chile (30°–39° S). Fire weather conditions (including high temperatures, low humidity, dryness, and strong winds) increase the potential for wildfires, once ignited, to rapidly spread. We show that the concurrence of El Niño and climate-fueled droughts and heatwaves boost the local fire risk and have decisively contributed to the intense fire activity recently seen in Central Chile. Our results also suggest that the tropical eastern Pacific Ocean variability modulates the seasonal fire weather in the country, driving in turn the interannual fire activity. The signature of the warm anomalies in the Niño 1 + 2 region (0°–10° S, 90° W–80° W) is apparent on the burned area records seen in Central Chile in 2017 and 2023.

DOI: https://doi.org/10.1038/s41598-024-52481-x

Fig. 1. A severe drought worsened by persistent heatwaves fueled fierce fires in February 2023 in Central Chile. (a) Precipitation for February 2023 relative to the 1981–2010 mean. The dry February 2023 came on top of the megadrought that has affected central Chile since 2008. (b) Air temperature for February 2023 relative to the 1981–2010 mean. February 2023 was the warmest on record in Central Chile. (c) Fire Weather Index (FWI) for February 2023 relative to the 1981–2010 mean. Extreme anomalies were registered in the regions severely affected by fires. (d) False-color image acquired on 3 February 2023 by the Operational Land Imager (OLI) on Landsat 8 showing the burn scar of Santa Juana Fire, in the BioBio Region, 100 km southeast of Concepcion, the second most populated city in the country.

New paper on urban waste production published in Nature Cities

Our new paper, “Worldwide scaling of waste generation in urban systems“, is published in Nature Cities.

The paper and its supporting information can be downloaded at https://www.nature.com/articles/s44284-023-00021-5. Data collected and compiled in this study are available in the figshare repository: https://doi.org/10.6084/m9.figshare.19361675.

Authors: Mingzhen Lu, Chuanbin Zhou, Chenghao Wang, Robert B. Jackson, Christopher P. Kempes

Abstract: The production of waste as a consequence of human activities is one of the most fundamental challenges facing our society and global ecological systems. Waste generation is rapidly increasing, with corresponding shifts in the structure of our societies, where almost all nations are moving from rural agrarian societies to urban and technological ones. However, the connections between these societal shifts and waste generation have not yet been described. In this study we applied scaling theory to establish a new understanding of waste in urban systems and identified universal scaling laws of waste generation across diverse urban systems worldwide for three forms of waste: wastewater, municipal solid waste, and greenhouse gases. We found that wastewater generation scales superlinearly, municipal solid waste scales linearly, and greenhouse gas emissions scale sublinearly with city size. In specific cases, production can be understood in terms of city size coupled with financial and natural resources. For example, wastewater generation can be understood in terms of the increased economic activity of larger cities, and the deviations from the scaling relationship, indicating relative efficiency, depend on gross domestic product per person and local rainfall. The temporal evolution of these scaling relationships reveals a loss of economies of scale and a general increase in waste production, where sublinear scaling relationships become linear. Our findings suggest general mechanisms controlling waste generation across diverse cities and global urban systems. Our approach offers a systematic framework to uncover these underlying mechanisms that might be key to reducing waste and pursuing a more sustainable future.

DOI: https://doi.org/10.1038/s44284-023-00021-5

Fig. 1. Scaling law of waste production across cities worldwide. a, Geolocation of the cities included in this study from three distinct data sources. MoHURD, Ministry of Housing and Urban Rural Development (China). The map was generated using R with the ‘ggplot2’ package. b, Wastewater production scales superlinearly with the size of cities (β = 1.15 ± 0.04, n = 675). We highlight two example cities (black circles) that stand out with a large deviation from the scaling law. Dongguan, an industrial city of southern China that features high personal wealth and high annual precipitation, generates disproportionately more wastewater than expected given its size. In contrast, the northwestern city of Tianshui, which features much lower personal wealth and rainfall, generates much less wastewater than expected given its size. c, MSW production scales linearly with city size (β = 1.04 ± 0.05, n = 292). We highlight Seattle (United States) and Lilongwe (Malawi) as two cities that deviate from the general scaling relationship. The much richer Seattle produces eight times more municipal waste than Lilongwe, even though it has a smaller population. d, The emission of GHGs displays sublinear scaling across cities worldwide (β = 0.85 ± 0.1, n = 296). We highlight Rotterdam (the Netherlands) and Bandung (Indonesia) as two cities that deviate from the general scaling relationship, with Rotterdam producing disproportionately more GHGs. The purpose of highlighting certain high- and low-residual cities is to give concrete examples so that readers can relate to the abstract data points presented here (no subjective judgements are made here). The dark gray error bands in bd represent the CIs of each scaling relationship.

New paper on N2O emissions from urban wastewater-influenced estuaries published in Communications Earth & Environment

Our new paper, “Wastewater-influenced estuaries are characterized by disproportionately high nitrous oxide emissions but overestimated IPCC emission factor“, is published in Communications Earth & Environment (IF: 7.9).

The paper and its supporting information can be downloaded at https://www.nature.com/articles/s43247-023-01051-6. Data collected and compiled in this study are available in the figshare repository: https://doi.org/10.6084/m9.figshare.24129774.

Authors: Yue Dong, Jia Liu, Xiang Cheng, Fuqiang Fan, Wei Lin, Chunyang Zhou, Shengrui Wang, Shangbin Xiao, Chenghao Wang, Yu Li, and Changlin Li

Abstract: Estuaries play an important role in the global nitrous oxide budget. However, considerable uncertainties exist in estimating their nitrous oxide emissions, largely due to anthropogenic impacts, particularly wastewater discharge. Here we investigate nitrous oxide emission dynamics in the Pearl River Estuary through advanced high-resolution, real-time measurements. Results suggest that Pearl River Estuary is a strong nitrous oxide emission source (1.05 Gg yr−1; range: 0.92–1.23 Gg yr−1) with pronounced spatial heterogeneity. Wastewater discharge substantially impacts emissions by introducing abundant nutrients, altering carbon-to-nitrogen stoichiometry, and stimulating biochemical processes. A meta-analysis further reveals the widespread enhancement of nitrous oxide emission induced by wastewater nitrogen input in global estuaries, with nitrous oxide emission factors considerably lower than that suggested by the IPCC owing to progressive biological saturation. Consequently, refining emission factor estimates through comprehensive bottom-up studies is imperative to improve the understanding of estuarine contributions to the global nitrous oxide budget.

DOI: https://doi.org/10.1038/s43247-023-01051-6

Fig. 2. Spatial distribution of N2O concentrations, saturations, and air–water fluxes in the Pearl River Estuary. a Dissolved N2O concentrations. b N2O saturations. c N2O fluxes. Spatial distributions were interpolated from high-resolution, real-time data using Kriging interpolation. The yellow box in (a) indicates the N2O concentration hotspot to the northwest of Inner Lingding Island.

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